During the 1950s, Lorenz became skeptical of the appropriateness of the linear statistical models in meteorology, as most atmospheric phenomena involved in weather forecasting are non-linear.[2] His work on the topic culminated in the publication of his 1963 paper "Deterministic Nonperiodic Flow" in Journal of the Atmospheric Sciences, and with it, the foundation of chaos theory.[2][5][6] He states in that paper:

Two states differing by imperceptible amounts may eventually evolve into two considerably different states ... If, then, there is any error whatever in observing the present state—and in any real system such errors seem inevitable—an acceptable prediction of an instantaneous state in the distant future may well be impossible....In view of the inevitable inaccuracy and incompleteness of weather observations, precise very-long-range forecasting would seem to be nonexistent.

His description of the butterfly effect followed in 1969.[2][7][8] He was awarded the Kyoto Prize for basic sciences, in the field of earth and planetary sciences, in 1991,[9] the Buys Ballot Award in 2004, and the Tomassoni Award in 2008. [10]